Systematic screening of gas diffusion layers for high performance CO2 electrolysis

Certain industrially relevant performance metrics of CO 2 electrolyzers have already been approached in recent years. The energy efficiency of CO 2 electrolyzers, however, is yet to be improved, and the reasons behind performance fading must be uncovered. The performance of the electrolyzer cells is...

Teljes leírás

Elmentve itt :
Bibliográfiai részletek
Szerzők: Samu Angelika Anita
Szenti Imre
Kukovecz Ákos
Endrődi Balázs
Janáky Csaba
Dokumentumtípus: Cikk
Megjelent: 2023
Sorozat:COMMUNICATIONS CHEMISTRY 6 No. 1
Tárgyszavak:
doi:10.1038/s42004-023-00836-2

mtmt:33708159
Online Access:http://publicatio.bibl.u-szeged.hu/27718
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520 3 |a Certain industrially relevant performance metrics of CO 2 electrolyzers have already been approached in recent years. The energy efficiency of CO 2 electrolyzers, however, is yet to be improved, and the reasons behind performance fading must be uncovered. The performance of the electrolyzer cells is strongly affected by their components, among which the gas diffusion electrode is one of the most critical elements. To understand which parameters of the gas diffusion layers (GDLs) affect the cell performance the most, we compared commercially available GDLs in the electrochemical reduction of CO 2 to CO, under identical, fully controlled experimental conditions. By systematically screening the most frequently used GDLs and their counterparts differing in only one parameter, we tested the influence of the microporous layer, the polytetrafluoroethylene content, the thickness, and the orientation of the carbon fibers of the GDLs. The electrochemical results were correlated to different physical/chemical parameters of the GDLs, such as their hydrophobicity and surface cracking. 
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700 0 1 |a Kukovecz Ákos  |e aut 
700 0 1 |a Endrődi Balázs  |e aut 
700 0 1 |a Janáky Csaba  |e aut 
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